Elucidating reaction dynamics in lithium–sulfur batteries via operando X-ray diffraction of hollow carbon sphere hosts

Abstract Lithium–sulfur (Li–S) batteries offer a promising route to affordable, clean, and high-performance energy storage. However, their widespread adoption is hindered by complex and inefficient charge storage mechanisms. Hollow carbon spheres have demonstrated improved Li–S cell performance, yet...

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Main Authors: Deaglán Bowman, Erlantz Lizundia, David McNulty
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Communications Materials
Online Access:https://doi.org/10.1038/s43246-025-00883-3
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author Deaglán Bowman
Erlantz Lizundia
David McNulty
author_facet Deaglán Bowman
Erlantz Lizundia
David McNulty
author_sort Deaglán Bowman
collection DOAJ
description Abstract Lithium–sulfur (Li–S) batteries offer a promising route to affordable, clean, and high-performance energy storage. However, their widespread adoption is hindered by complex and inefficient charge storage mechanisms. Hollow carbon spheres have demonstrated improved Li–S cell performance, yet their specific effect on sulfur/Li2S conversion dynamics remains insufficiently understood. Here, we present a facile synthesis method for glucose-derived hollow carbon spheres, delivering a high specific charge of 1159 mAh g−1 (C/10) and a reversible specific charge of 510 mAh g−1 after 500 cycles (C/5). Using operando X-ray diffraction, we investigate their influence on Li–S reaction dynamics. Analysis of relative peak intensities and full width at half-maximum indicates a plateau in Li2S crystallite size at 60% depth of discharge. This supports the formation of a disproportionation-driven amorphous polysulphide matrix that restricts Li2S crystallite growth and discharge capacity. Electro-crystallisation induces notable changes to sulfur upon charge, including shifts in allotropes and crystallite orientation.
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spelling doaj-art-06befe4bfdb0463799e33a814abb83ea2025-08-20T03:46:28ZengNature PortfolioCommunications Materials2662-44432025-07-016111310.1038/s43246-025-00883-3Elucidating reaction dynamics in lithium–sulfur batteries via operando X-ray diffraction of hollow carbon sphere hostsDeaglán Bowman0Erlantz Lizundia1David McNulty2Department of Chemical Sciences and Bernal Institute, University of LimerickLife Cycle Thinking Group, Department of Graphic Design and Engineering Projects, University of the Basque Country (UPV/EHU)Department of Physics and Bernal Institute, University of LimerickAbstract Lithium–sulfur (Li–S) batteries offer a promising route to affordable, clean, and high-performance energy storage. However, their widespread adoption is hindered by complex and inefficient charge storage mechanisms. Hollow carbon spheres have demonstrated improved Li–S cell performance, yet their specific effect on sulfur/Li2S conversion dynamics remains insufficiently understood. Here, we present a facile synthesis method for glucose-derived hollow carbon spheres, delivering a high specific charge of 1159 mAh g−1 (C/10) and a reversible specific charge of 510 mAh g−1 after 500 cycles (C/5). Using operando X-ray diffraction, we investigate their influence on Li–S reaction dynamics. Analysis of relative peak intensities and full width at half-maximum indicates a plateau in Li2S crystallite size at 60% depth of discharge. This supports the formation of a disproportionation-driven amorphous polysulphide matrix that restricts Li2S crystallite growth and discharge capacity. Electro-crystallisation induces notable changes to sulfur upon charge, including shifts in allotropes and crystallite orientation.https://doi.org/10.1038/s43246-025-00883-3
spellingShingle Deaglán Bowman
Erlantz Lizundia
David McNulty
Elucidating reaction dynamics in lithium–sulfur batteries via operando X-ray diffraction of hollow carbon sphere hosts
Communications Materials
title Elucidating reaction dynamics in lithium–sulfur batteries via operando X-ray diffraction of hollow carbon sphere hosts
title_full Elucidating reaction dynamics in lithium–sulfur batteries via operando X-ray diffraction of hollow carbon sphere hosts
title_fullStr Elucidating reaction dynamics in lithium–sulfur batteries via operando X-ray diffraction of hollow carbon sphere hosts
title_full_unstemmed Elucidating reaction dynamics in lithium–sulfur batteries via operando X-ray diffraction of hollow carbon sphere hosts
title_short Elucidating reaction dynamics in lithium–sulfur batteries via operando X-ray diffraction of hollow carbon sphere hosts
title_sort elucidating reaction dynamics in lithium sulfur batteries via operando x ray diffraction of hollow carbon sphere hosts
url https://doi.org/10.1038/s43246-025-00883-3
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