A New Decavanadate with Organic Cation: Synthesis, Crystal Structure, and Hirshfeld Surface Analysis

A new 2,6-bis aminomethyl piperidine decavanadate hydrate, (C7N3H20)2V10O28.4.21H2O, was synthesized by slow evaporation of a solution at room temperature. The molecular structure was investigated by single-crystal X-ray diffraction. In the crystal structure, the layers of decavanadate groups, organ...

Full description

Saved in:
Bibliographic Details
Main Authors: Rawia Nasri, Regaya Ksiksi, Mohsen Graia, Mohamed Faouzi Zid
Format: Article
Language:English
Published: Wiley 2021-01-01
Series:Advances in Materials Science and Engineering
Online Access:http://dx.doi.org/10.1155/2021/5542315
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850233364936654848
author Rawia Nasri
Regaya Ksiksi
Mohsen Graia
Mohamed Faouzi Zid
author_facet Rawia Nasri
Regaya Ksiksi
Mohsen Graia
Mohamed Faouzi Zid
author_sort Rawia Nasri
collection DOAJ
description A new 2,6-bis aminomethyl piperidine decavanadate hydrate, (C7N3H20)2V10O28.4.21H2O, was synthesized by slow evaporation of a solution at room temperature. The molecular structure was investigated by single-crystal X-ray diffraction. In the crystal structure, the layers of decavanadate groups, organic cations, and water molecules are arranged parallel to the (010) plane. Also, the prepared compound has been analysed by FTIR spectroscopy and scanning electron microscopy (SEM). The crystal structure of the title compound is stabilized by hydrogen bonds and van der Waals interactions. The cohesion of the structure is ensured by O-H…O and N-H…O hydrogen bonds. The three-dimensional Hirshfeld surface (3D-HS) and the relative two-dimensional fingerprint plots (2D-FPs) of (C7N3H20)2V10O28.4.21H2O compound revealed that the structure is dominated by O…H/H…O (70.8%) and H…H (18.5%) contacts.
format Article
id doaj-art-05bbcecdcd334d39a249a0f92a447366
institution OA Journals
issn 1687-8434
1687-8442
language English
publishDate 2021-01-01
publisher Wiley
record_format Article
series Advances in Materials Science and Engineering
spelling doaj-art-05bbcecdcd334d39a249a0f92a4473662025-08-20T02:02:57ZengWileyAdvances in Materials Science and Engineering1687-84341687-84422021-01-01202110.1155/2021/55423155542315A New Decavanadate with Organic Cation: Synthesis, Crystal Structure, and Hirshfeld Surface AnalysisRawia Nasri0Regaya Ksiksi1Mohsen Graia2Mohamed Faouzi Zid3University of Tunis El Manar, Faculty of Sciences of Tunis, Laboratory of Materials, Crystal Chemistry and Applied Thermodynamics, 2092 El Manar II, Tunis, TunisiaUniversity of Tunis El Manar, Faculty of Sciences of Tunis, Laboratory of Materials, Crystal Chemistry and Applied Thermodynamics, 2092 El Manar II, Tunis, TunisiaFaculty of Sciences of Sfax, Solid State Laboratory, Faculty of Sciences, University of Sfax, 1171 Sfax 3000, TunisiaUniversity of Tunis El Manar, Faculty of Sciences of Tunis, Laboratory of Materials, Crystal Chemistry and Applied Thermodynamics, 2092 El Manar II, Tunis, TunisiaA new 2,6-bis aminomethyl piperidine decavanadate hydrate, (C7N3H20)2V10O28.4.21H2O, was synthesized by slow evaporation of a solution at room temperature. The molecular structure was investigated by single-crystal X-ray diffraction. In the crystal structure, the layers of decavanadate groups, organic cations, and water molecules are arranged parallel to the (010) plane. Also, the prepared compound has been analysed by FTIR spectroscopy and scanning electron microscopy (SEM). The crystal structure of the title compound is stabilized by hydrogen bonds and van der Waals interactions. The cohesion of the structure is ensured by O-H…O and N-H…O hydrogen bonds. The three-dimensional Hirshfeld surface (3D-HS) and the relative two-dimensional fingerprint plots (2D-FPs) of (C7N3H20)2V10O28.4.21H2O compound revealed that the structure is dominated by O…H/H…O (70.8%) and H…H (18.5%) contacts.http://dx.doi.org/10.1155/2021/5542315
spellingShingle Rawia Nasri
Regaya Ksiksi
Mohsen Graia
Mohamed Faouzi Zid
A New Decavanadate with Organic Cation: Synthesis, Crystal Structure, and Hirshfeld Surface Analysis
Advances in Materials Science and Engineering
title A New Decavanadate with Organic Cation: Synthesis, Crystal Structure, and Hirshfeld Surface Analysis
title_full A New Decavanadate with Organic Cation: Synthesis, Crystal Structure, and Hirshfeld Surface Analysis
title_fullStr A New Decavanadate with Organic Cation: Synthesis, Crystal Structure, and Hirshfeld Surface Analysis
title_full_unstemmed A New Decavanadate with Organic Cation: Synthesis, Crystal Structure, and Hirshfeld Surface Analysis
title_short A New Decavanadate with Organic Cation: Synthesis, Crystal Structure, and Hirshfeld Surface Analysis
title_sort new decavanadate with organic cation synthesis crystal structure and hirshfeld surface analysis
url http://dx.doi.org/10.1155/2021/5542315
work_keys_str_mv AT rawianasri anewdecavanadatewithorganiccationsynthesiscrystalstructureandhirshfeldsurfaceanalysis
AT regayaksiksi anewdecavanadatewithorganiccationsynthesiscrystalstructureandhirshfeldsurfaceanalysis
AT mohsengraia anewdecavanadatewithorganiccationsynthesiscrystalstructureandhirshfeldsurfaceanalysis
AT mohamedfaouzizid anewdecavanadatewithorganiccationsynthesiscrystalstructureandhirshfeldsurfaceanalysis
AT rawianasri newdecavanadatewithorganiccationsynthesiscrystalstructureandhirshfeldsurfaceanalysis
AT regayaksiksi newdecavanadatewithorganiccationsynthesiscrystalstructureandhirshfeldsurfaceanalysis
AT mohsengraia newdecavanadatewithorganiccationsynthesiscrystalstructureandhirshfeldsurfaceanalysis
AT mohamedfaouzizid newdecavanadatewithorganiccationsynthesiscrystalstructureandhirshfeldsurfaceanalysis