Optical Characterization of Fluorescent Chitosan-Based Carbon Dots Embedded in Aqueous Natural Dye

(1) Background: This work evaluated the optical characterization of aqueous fluorescent chitosan-based carbon dots (or carbon nanoparticles CNPs) embedded in natural dye for potential functional packaging applications. Chitosan-based materials are nontoxic, biodegradable, biocompatible, bactericidal...

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Bibliographic Details
Main Authors: Sthanley R. De Lima, Thiago V. Costa, Tácio T. S. Santos, Dora G. Felipe, Teófanes B. Serna, Acácio A. Andrade, Viviane Pilla
Format: Article
Language:English
Published: MDPI AG 2024-10-01
Series:Colorants
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Online Access:https://www.mdpi.com/2079-6447/3/4/19
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Summary:(1) Background: This work evaluated the optical characterization of aqueous fluorescent chitosan-based carbon dots (or carbon nanoparticles CNPs) embedded in natural dye for potential functional packaging applications. Chitosan-based materials are nontoxic, biodegradable, biocompatible, bactericidal, and produced from renewable polymer sources. Anthocyanins are pigments of different colors with a large range of potential applications, such as in bioindicators and biomonitoring; (2) Methods: The CNPs were synthetized in aqueous solutions using chitosan as a carbon source. The natural dye was extracted from the leaves of <i>Tradescantia pallida</i> Purpurea in aqueous solutions. The fluorescence quantum efficiency (η) and fluorescence lifetime (τ) were determined using the mode-mismatched pump–probe thermal lens (TL) technique and time-resolved fluorescence lifetimes (TRFL) measurements, respectively; (3) Results: The η and τ were measured for CNPs embedded in natural dye solution at different concentrations (5.2, 12.09, and 21.57 mass percentage composition). The η and τ photophysical parameters obtained for CNPs embedded in natural dye were compared with those of other CNPs synthesized using different carbon sources, such as leaves, seeds, and protein; (4) Conclusions: Fluorescence spectra and time-resolved fluorescence measurements corroborate the TL results, and relatively high values of η were obtained for the CNP synthesized and embedded in natural dye.
ISSN:2079-6447