Computational generation of tailored radionuclide libraries for alpha-particle and gamma-ray spectrometry
Radionuclide identification is a radioanalytical method employed in various scientific disciplines that utilize alpha-particle or gamma-ray spectrometric assays, ranging from astrophysics to nuclear medicine. Radionuclide libraries in conventional radionuclide identification systems are crafted in a...
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| Main Author: | |
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| Format: | Article |
| Language: | English |
| Published: |
American Physical Society
2024-11-01
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| Series: | Physical Review Research |
| Online Access: | http://doi.org/10.1103/PhysRevResearch.6.043208 |
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| Summary: | Radionuclide identification is a radioanalytical method employed in various scientific disciplines that utilize alpha-particle or gamma-ray spectrometric assays, ranging from astrophysics to nuclear medicine. Radionuclide libraries in conventional radionuclide identification systems are crafted in a manual fashion, accompanying labor-intensive and error-prone user tasks and hindering library customization. This research presents a computational algorithm and the architecture of its dedicated software that can automatically generate tailored radionuclide libraries. Progenitor-progeny recurrence relations were modeled to enable recursive computation of radionuclide subsets. This theoretical concept was incorporated into open-source software called RecurLib and validated against four actinide decay series and 12 radioactive substances, including a uranium-glazed legacy Fiestaware, natural uranium and thorium sources, a ^{226}Ra sample, and the medical radionuclides ^{225}Ac, ^{177}Lu, and ^{99m}Tc. The developed algorithm yielded radionuclide libraries for all the tested specimens within minutes, demonstrating its efficiency and applicability across diverse scenarios. The proposed approach introduces a framework for computerized radionuclide library generation, thereby trivializing library-driven radionuclide identification and facilitating the spectral recognition of unregistered radionuclides in radiation spectrometry. |
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| ISSN: | 2643-1564 |