Dynamic Assembly of Microgels and Polymers at Non‐Aqueous Liquid/Liquid Interfaces

Abstract Particle assembly at liquid–liquid interfaces presents a promising bottom‐up strategy for creating supramolecular materials with advanced functionalities. However, the significantly lower interfacial tension observed in immiscible organic phases compared to traditional oil–water systems has...

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Main Authors: Xin Guan, Yang Liu, Lianwei Li, Man‐Hin Kwok, Mingming Ding, Hang Jiang, To Ngai
Format: Article
Language:English
Published: Wiley 2025-04-01
Series:Advanced Science
Subjects:
Online Access:https://doi.org/10.1002/advs.202415642
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author Xin Guan
Yang Liu
Lianwei Li
Man‐Hin Kwok
Mingming Ding
Hang Jiang
To Ngai
author_facet Xin Guan
Yang Liu
Lianwei Li
Man‐Hin Kwok
Mingming Ding
Hang Jiang
To Ngai
author_sort Xin Guan
collection DOAJ
description Abstract Particle assembly at liquid–liquid interfaces presents a promising bottom‐up strategy for creating supramolecular materials with advanced functionalities. However, the significantly lower interfacial tension observed in immiscible organic phases compared to traditional oil–water systems has hindered the effective adsorption and assembly of particles at oil–oil interfaces. In this work, a versatile and effective strategy is presented that utilizes the assembly and jamming of microgels and polymer ligands at non‐aqueous liquid–liquid interfaces to create non‐aqueous Pickering emulsions and reconfigurable droplet networks. The resulting microgel‐polymer complexes form an asymmetric interfacial bilayer with high surface coverage, which effectively minimizes interfacial energy and improves interfacial elasticity. Through a combination of systematic interfacial measurements and molecular dynamics simulations, the underlying mechanisms governing interfacial self‐assembly are elucidated. Notably, the stimuli‐responsive nature of the microgel‐polymer complexes allows for precise control over the interfacial assembly and disassembly by introducing competitive molecules. Furthermore, it is demonstrated that these non‐aqueous Pickering emulsions serve as excellent templates for the fabrication of heterogeneous organogels and microgel‐based colloidosomes through both covalent and non‐covalent crosslinking strategies. This work underscores the potential of non‐aqueous interfaces in advancing materials science and opens new avenues for developing multifunctional materials.
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issn 2198-3844
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spelling doaj-art-003064a48b75415db1cfab0acfcee5b22025-08-20T01:51:39ZengWileyAdvanced Science2198-38442025-04-011213n/an/a10.1002/advs.202415642Dynamic Assembly of Microgels and Polymers at Non‐Aqueous Liquid/Liquid InterfacesXin Guan0Yang Liu1Lianwei Li2Man‐Hin Kwok3Mingming Ding4Hang Jiang5To Ngai6Department of Chemistry The Chinese University of Hong Kong Shatin, N.T Hong Kong ChinaCollege of Polymer Science and Engineering State Key Laboratory of Polymer Materials Engineering Sichuan University Chengdu 610065 ChinaCollege of Chemistry and Environmental Engineering Shenzhen University Shenzhen 518060 ChinaDepartment of Chemistry The Chinese University of Hong Kong Shatin, N.T Hong Kong ChinaCollege of Polymer Science and Engineering State Key Laboratory of Polymer Materials Engineering Sichuan University Chengdu 610065 ChinaKey Laboratory of Synthetic and Biological Colloids Ministry of Education & School of Chemical and Material Engineering Jiangnan University Wuxi 214122 ChinaDepartment of Chemistry The Chinese University of Hong Kong Shatin, N.T Hong Kong ChinaAbstract Particle assembly at liquid–liquid interfaces presents a promising bottom‐up strategy for creating supramolecular materials with advanced functionalities. However, the significantly lower interfacial tension observed in immiscible organic phases compared to traditional oil–water systems has hindered the effective adsorption and assembly of particles at oil–oil interfaces. In this work, a versatile and effective strategy is presented that utilizes the assembly and jamming of microgels and polymer ligands at non‐aqueous liquid–liquid interfaces to create non‐aqueous Pickering emulsions and reconfigurable droplet networks. The resulting microgel‐polymer complexes form an asymmetric interfacial bilayer with high surface coverage, which effectively minimizes interfacial energy and improves interfacial elasticity. Through a combination of systematic interfacial measurements and molecular dynamics simulations, the underlying mechanisms governing interfacial self‐assembly are elucidated. Notably, the stimuli‐responsive nature of the microgel‐polymer complexes allows for precise control over the interfacial assembly and disassembly by introducing competitive molecules. Furthermore, it is demonstrated that these non‐aqueous Pickering emulsions serve as excellent templates for the fabrication of heterogeneous organogels and microgel‐based colloidosomes through both covalent and non‐covalent crosslinking strategies. This work underscores the potential of non‐aqueous interfaces in advancing materials science and opens new avenues for developing multifunctional materials.https://doi.org/10.1002/advs.202415642interfacial assemblyliquid structuringmicrogel‐polymer complexesorganogelsPickering emulsions
spellingShingle Xin Guan
Yang Liu
Lianwei Li
Man‐Hin Kwok
Mingming Ding
Hang Jiang
To Ngai
Dynamic Assembly of Microgels and Polymers at Non‐Aqueous Liquid/Liquid Interfaces
Advanced Science
interfacial assembly
liquid structuring
microgel‐polymer complexes
organogels
Pickering emulsions
title Dynamic Assembly of Microgels and Polymers at Non‐Aqueous Liquid/Liquid Interfaces
title_full Dynamic Assembly of Microgels and Polymers at Non‐Aqueous Liquid/Liquid Interfaces
title_fullStr Dynamic Assembly of Microgels and Polymers at Non‐Aqueous Liquid/Liquid Interfaces
title_full_unstemmed Dynamic Assembly of Microgels and Polymers at Non‐Aqueous Liquid/Liquid Interfaces
title_short Dynamic Assembly of Microgels and Polymers at Non‐Aqueous Liquid/Liquid Interfaces
title_sort dynamic assembly of microgels and polymers at non aqueous liquid liquid interfaces
topic interfacial assembly
liquid structuring
microgel‐polymer complexes
organogels
Pickering emulsions
url https://doi.org/10.1002/advs.202415642
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AT mingmingding dynamicassemblyofmicrogelsandpolymersatnonaqueousliquidliquidinterfaces
AT hangjiang dynamicassemblyofmicrogelsandpolymersatnonaqueousliquidliquidinterfaces
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