Structure and Spatial Distribution of Ge Nanocrystals Subjected to Fast Neutron Irradiation

The influence of fast neutron irradiation on the structure and spatial distribution of Ge nanocrystals (NC) embedded in an amorphous SiO2 matrix has been studied. The investigation was conducted by means of laser Raman Scattering (RS), High Resolution Transmission Electron Microscopy (HR-TEM) and X-...

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Main Authors: Alexander N. Ionov, Tiecheng Lu, Yossi Gofer, Judith Grinblat, David H. Dressler, Issai Shlimak, Shai Levy
Format: Article
Language:English
Published: Wiley 2011-07-01
Series:Nanomaterials and Nanotechnology
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Online Access:http://www.intechopen.com/journals/nanomaterials_and_nanotechnology/structure_and_spatial_distribution_of_ge_nanocrystals_subjected_to_fast_neutron_irradiation
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author Alexander N. Ionov
Tiecheng Lu
Yossi Gofer
Judith Grinblat
David H. Dressler
Issai Shlimak
Shai Levy
author_facet Alexander N. Ionov
Tiecheng Lu
Yossi Gofer
Judith Grinblat
David H. Dressler
Issai Shlimak
Shai Levy
author_sort Alexander N. Ionov
collection DOAJ
description The influence of fast neutron irradiation on the structure and spatial distribution of Ge nanocrystals (NC) embedded in an amorphous SiO2 matrix has been studied. The investigation was conducted by means of laser Raman Scattering (RS), High Resolution Transmission Electron Microscopy (HR-TEM) and X-ray photoelectron spectroscopy (XPS). The irradiation of Ge- NC samples by a high dose of fast neutrons lead to a partial destruction of the nanocrystals. Full reconstruction of crystallinity was achieved after annealing the radiation damage at 8000C, which resulted in full restoration of the RS spectrum. HR-TEM images show, however, that the spatial distributions of Ge-NC changed as a result of irradiation and annealing. A sharp decrease in NC distribution towards the SiO2 surface has been observed. This was accompanied by XPS detection of Ge oxides and elemental Ge within both the surface and subsurface region.
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publishDate 2011-07-01
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series Nanomaterials and Nanotechnology
spelling doaj-art-000ec79f889b4b739ac15856929b0d2e2025-08-20T02:03:14ZengWileyNanomaterials and Nanotechnology1847-98042011-07-0111http://dx.doi.org/10.5772/50951Structure and Spatial Distribution of Ge Nanocrystals Subjected to Fast Neutron IrradiationAlexander N. IonovTiecheng LuYossi GoferJudith GrinblatDavid H. DresslerIssai ShlimakShai LevyThe influence of fast neutron irradiation on the structure and spatial distribution of Ge nanocrystals (NC) embedded in an amorphous SiO2 matrix has been studied. The investigation was conducted by means of laser Raman Scattering (RS), High Resolution Transmission Electron Microscopy (HR-TEM) and X-ray photoelectron spectroscopy (XPS). The irradiation of Ge- NC samples by a high dose of fast neutrons lead to a partial destruction of the nanocrystals. Full reconstruction of crystallinity was achieved after annealing the radiation damage at 8000C, which resulted in full restoration of the RS spectrum. HR-TEM images show, however, that the spatial distributions of Ge-NC changed as a result of irradiation and annealing. A sharp decrease in NC distribution towards the SiO2 surface has been observed. This was accompanied by XPS detection of Ge oxides and elemental Ge within both the surface and subsurface region.http://www.intechopen.com/journals/nanomaterials_and_nanotechnology/structure_and_spatial_distribution_of_ge_nanocrystals_subjected_to_fast_neutron_irradiation Ge nanocrystalsNeutron radiation effectsStructure and spatial distribution
spellingShingle Alexander N. Ionov
Tiecheng Lu
Yossi Gofer
Judith Grinblat
David H. Dressler
Issai Shlimak
Shai Levy
Structure and Spatial Distribution of Ge Nanocrystals Subjected to Fast Neutron Irradiation
Nanomaterials and Nanotechnology
Ge nanocrystals
Neutron radiation effects
Structure and spatial distribution
title Structure and Spatial Distribution of Ge Nanocrystals Subjected to Fast Neutron Irradiation
title_full Structure and Spatial Distribution of Ge Nanocrystals Subjected to Fast Neutron Irradiation
title_fullStr Structure and Spatial Distribution of Ge Nanocrystals Subjected to Fast Neutron Irradiation
title_full_unstemmed Structure and Spatial Distribution of Ge Nanocrystals Subjected to Fast Neutron Irradiation
title_short Structure and Spatial Distribution of Ge Nanocrystals Subjected to Fast Neutron Irradiation
title_sort structure and spatial distribution of ge nanocrystals subjected to fast neutron irradiation
topic Ge nanocrystals
Neutron radiation effects
Structure and spatial distribution
url http://www.intechopen.com/journals/nanomaterials_and_nanotechnology/structure_and_spatial_distribution_of_ge_nanocrystals_subjected_to_fast_neutron_irradiation
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AT judithgrinblat structureandspatialdistributionofgenanocrystalssubjectedtofastneutronirradiation
AT davidhdressler structureandspatialdistributionofgenanocrystalssubjectedtofastneutronirradiation
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